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  • Applications of Holographic Optical Tweezers: Multiplexed Fluorescence Spectroscopy and the Micromechanics of Type-I Collagen

    Creator:
    Cibula, Matthew A.
    Abstract:
    The development and some applications of holographic optical tweezers (HOT) are presented. Our HOT system uses a spatial light modulator (SLM) to control the location and properties of the optical trap. We have developed a method for optimizing the diffraction efficiency of a SLM that can be applied in situ...
    Resource Type:
    Dissertation
    Full Text:
    Type-I Collagen Abstract approved: David H. McIntyre The development and some applications of

  • CoLocalized Excitation Emission Resolution : A CLEER approach for multicolor fluorescence analysis

    Creator:
    Almlie, C. Kyle
    Abstract:
    Fluorescence has proven to be a robust and powerful method of analysis in numerous fields: forensics, pharmaceutics, geology, food science, and environmental sciences have all developed a large collection of fluorescence instruments and methods to overcome application-specific challenges. Biological applications saw the same development of a fluorescence toolkit with methods...
    Resource Type:
    Dissertation
    Full Text:
    for the degree of Doctor of Philosophy in Chemistry presented on June 27, 2017. Title: CoLocalized

  • Liquid-gated carbon nanotube transistor noise sources and sensitivity limits

    Creator:
    Sharf, Tal
    Abstract:
    Low-dimensional electronic materials offer a platform to observe biological processes with unprecedented spatial and temporal resolution. Carbon nanotubes (CNTs) are the closest physical analog to an ideal 1D system and can be scaled and integrated into multiplexed electronic circuitry. The molecular structure of a CNT is also biocompatible, making them...
    Resource Type:
    Dissertation
    Full Text:
    August 27, 2014. Title: Liquid-Gated Carbon Nanotube Transistor Noise Sources and Sensitivity

  • High-Field Terahertz Spectroscopy of Nanoscale Materials

    Creator:
    Mousavian, Ali
    Abstract:
    This dissertation covers my work relating to the application of strong terahertz (THz) radiation to study the nonlinear properties of nano-scale material. It presents experimental and numerical studies on the optical and electronic properties of various material system including single-layer graphene, multi-walled carbon nanotubes (MWCNTs), nanoantenna-patterned gallium arsenide (GaAs) and...
    Resource Type:
    Dissertation
    Full Text:
    pulses for time-domain pump-probe THz/optical spectroscopy. Due to the low photon energy (4 meV for

  • Terahertz Imaging and Nonlinear Spectroscopy of Semiconductors using Plasmonic Devices

    Creator:
    Thompson, Zachary James
    Abstract:
    In this dissertation, a series of studies in the field of terahertz (THz) science are presented, specifically using nonlinear THz spectroscopy. We exploit huge field enhancement and subwavelength confinement in plasmonic structures. There are three distinct projects which will be discussed: nonlinear THz spectroscopy using plasmonic induced transparency (PIT), THz-triggered...
    Resource Type:
    Dissertation
    Full Text:
    , a series of studies in the field of terahertz (THz) science are pre- sented, specifically using

  • BaCuChF (Ch = S, Se, Te) p-type transparent conductors

    Creator:
    Zakutayev, Andriy
    Abstract:
    BaCuChF (Ch = S, Se, Te) materials are chalcogen-based transparent conductors with wide optical band gaps (2.9 – 3.5 eV) and a high concentration of free holes (10¹⁸ – 10²⁰ cm⁻³) caused by the presence of copper vacancies. Chalcogen vacancies compensate copper vacancies in these materials, setting the Fermi level...
    Resource Type:
    Dissertation
    Full Text:
    27 A. Zakutayev, J. Tate, H. A. S. Platt, D. A. Keszler, C. Hein, T. Mayer, A. Klein, W

  • Electronic and Optical Properties of Defects in Amorphous Oxide and Transition Metal Dichalcogenide Semiconductors

    Creator:
    Vogt, Kyle
    Abstract:
    The optical and electronic properties of amorphous oxide thin films depend crucially on chemical composition, and deposition process variations which give rise to sub-gap defect states. Consequently, there is a need for a reliable, high-throughput method to extract sub-gap defect densities of states in amorphous oxide thin films. We present...
    Resource Type:
    Dissertation
    Full Text:
    respect to energy. The resulting fully- experimentally derived DoS reveals a series of broad defect peaks

  • Tracking Photoinduced Primary Events with Femtosecond Stimulated Raman Spectroscopy and Calculations

    Creator:
    Wang, Yanli
    Abstract:
    Femtosecond stimulated Raman spectroscopy (FSRS) is a powerful ultrafast technique which can track photoinduced excited state structural events on femtosecond (fs) to picosecond (ps) timescales. In addition to high temporal and spectral resolutions, FSRS provides a broad spectral window from ca. 100—2000 cm-1 for detection, enabling the direct mapping of...
    Resource Type:
    Dissertation
    Full Text:
    state photoacid (PA*) and photobase (PB*) forms of HPTS during ESPT. An intermolecular H-bond

  • Analysis of the mechanism of sulfoxide-lithium exchange and the reactive intermediate in stereospecific reagent-controlled homologation (StReCH)

    Creator:
    Hoyt, Amanda
    Abstract:
    The stereospecific reagent-controlled homologation (StReCH) of boronic esters with enantioenriched carbenoid species generated in situ by the addition of organolithium initiators to stereodefined α-chloroalkyl aryl sulfoxides was previously reported. The reaction of an organolithium with an α-chloroalkyl aryl sulfoxide ostensibly generates an α-chloroalkyllithium via sulfoxide-lithium exchange; however, the true nature...
    Resource Type:
    Masters Thesis
    Full Text:
    stirred in chloroform (55 mL) at rt for 2 h. Thioanisole 27 (2.64 mL, d = 1.057 g/mL, 2.79 g, 22.5

  • Study of creeping, inertial and turbulent flow regimes in porous media using particle image velocimetry

    Creator:
    Patil, Vishal A.
    Abstract:
    Porous media flows are encountered in many natural and man-made systems such as gas adsorption, filtration, heat exchangers, combustion, catalytic reactors and groundwater hydrology. This study experimentally investigates these flows as function of pore Reynolds number, Re[subscript pore]. The pore Reynolds number is based on the porous bed hydraulic diameter,...
    Resource Type:
    Dissertation
    Full Text:
    design, interpretation of data and writing of Chapter 2, 3, 4 and 5. TABLE OF CONTENTS