A new method for delayed gamma-ray spectrometry to quantify the relative content of fissile material is developed and demonstrated to support international efforts in bolstering non-destructive assay capabilities. Previous traditional delayed gamma-ray spectrometry techniques rely upon nuclear data that often carry very high uncertainty. The new method removes the requirement...
An integrated sampling and gamma ray spectrometry system has
been developed for analysis of TRIGA reactor primary cooling water.
A microcomputer controls pumps and valves using BASIC and assembly
language programs to pump 300 ml liquid samples into a reference
geometry surrounding a Ge(Li) detector. Gamma ray spectra are
acquired...
Perturbed Angular Correlation Spectroscopy (PAC) is a highly sensitive local
probe technique well suited for studying defect characteristics of solids. This technique is
applied to the problem of studying the solubility of indium in cerium oxide. Through the
measurement of samples with differing levels in indium doping, the solubility of...
Two applications of beta spectrometry using active
gamma-ray discrimination are described. The beta spectra
of smears taken at a nuclear power plant at the end of a
300 day shutdown were characterized. The average beta
energy at "contact" (1.5 cm) was between 450 and 550 keV
for locations influenced by...
The decay scheme of Mn⁵¹ has been investigated using gamma-ray
and beta-ray scintillation spectrometers and a fast coincidence
spectrometer. A half-life value of 46.5 ± 0.2 minutes was determined
for Mn⁵¹ which decays predominantly to the ground state of
Cr⁵¹ by the emission of positons with an experimentally measured
end-point...
During the past few decades, the U.S. Department of Energy (DOE) has made significant investments to improve nuclear data libraries, as the quality of this data impacts nearly all analyses of nuclear systems. Nuclear fission product yields are one component of these libraries, and are important for the analysis of...
Following thermal neutron induced fission, supervised machine learning and temporal gamma-ray spectroscopy methods were used to identify differences in the delayed gamma-ray spectra of Pu-239 and U-235. The temporal gamma-ray spectroscopy method takes advantage of the time-dependent decay of fission products. Employing Spearman's rank-order correlation coefficient and without prior knowledge...