RELATIVE INFLUENCE OF TRANS-PACIFIC AND REGIONAL ATMOSPHERIC TRANSPORT OF PAHS IN THE PACIFIC NORTHWEST, USA Public Deposited

http://ir.library.oregonstate.edu/concern/articles/wm117q87s

This is an author's in-press, peer-reviewed manuscript, as accepted by the publisher. The published article is copyrighted by the American Chemical Society and after publication, can be found at:  http://pubs.acs.org/journal/esthag

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  • The relative influences of trans-Pacific and regional atmospheric transport on measured concentrations of polycyclic aromatic hydrocarbons (PAHs), PAH derivatives [Nitro- (NPAH) and Oxy-(OPAH)], organic carbon (OC), and Particulate Matter (PM) less than 2.5 μm in diameter (PM₂.₅) were investigated in the Pacific Northwest, USA in 2010-2011. Ambient high volume PM₂.₅ air samples were collected at two sites in the Pacific Northwest: 1.) Mount Bachelor Observatory (MBO) in the Oregon Cascade Range (2763 m above sea level (asl)) and 2.) Confederated Tribes of the Umatilla Indian Reservation (CTUIR) in the Columbia River Gorge (CRG) (954 m asl). At MBO, the 1,8-dinitropyrene concentration was significantly positively correlated with the time a sampled air mass spent over Asia, suggesting that this NPAH may be a good marker for trans-Pacific atmospheric transport. At CTUIR, NOx, CO₂, and SO₂ emissions from a 585 MW coal fired power plant, in Boardman OR, were found to be significantly positively correlated with PAH, OPAH, NPAH, OC, and PM₂.₅ concentrations. By comparing the Boardman Plant operational time frames when the plant was operating to when it was shut down, the plant was found to contribute a large percentage of the measured PAH (67%), NPAH (91%), OPAH (54%), PM₂.₅ (39%) and OC (38%) concentrations at CTUIR and the CRG prior to Spring 2011 and likely masked trans-Pacific atmospheric transport events to the CRG. Upgrades installed to the Boardman Plant in the spring of 2011 dramatically reduced the plant’s contribution to PAH and OPAH concentrations (by ~72% and ~40%, respectively) at CTUIR and the CRG but not NPAH, PM₂.₅ or OC concentrations.
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  • Lafontaine, S., Schrlau, J., Butler, J., Jia, Y., Harper, B., Harris, S., … & Simonich, S. L. M. (2015). Relative Influence of Trans-Pacific and Regional Atmospheric Transport of PAHS in the Pacific Northwest, USA. [Article in Press]. Environmental Science & Technology.
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  • description.provenance : Approved for entry into archive by Deanne Bruner(deanne.bruner@oregonstate.edu) on 2015-07-06T19:23:30Z (GMT) No. of bitstreams: 2 SimonichStaciEnvironmentalMolecularToxicologyRelativeInfluenceTrans-Pacific.pdf: 2093385 bytes, checksum: cacc05da703959780798020d7f72cbbb (MD5) SimonichStaciEnvironmentalMolecularToxicologyRelativeInfluenceTrans-Pacific(SupportingInformation).pdf: 6448095 bytes, checksum: 86d0069afef09a4a7558a72ad3bc6d64 (MD5)
  • description.provenance : Made available in DSpace on 2015-07-06T19:23:30Z (GMT). No. of bitstreams: 2 SimonichStaciEnvironmentalMolecularToxicologyRelativeInfluenceTrans-Pacific.pdf: 2093385 bytes, checksum: cacc05da703959780798020d7f72cbbb (MD5) SimonichStaciEnvironmentalMolecularToxicologyRelativeInfluenceTrans-Pacific(SupportingInformation).pdf: 6448095 bytes, checksum: 86d0069afef09a4a7558a72ad3bc6d64 (MD5) Previous issue date: 2015
  • description.provenance : Submitted by Deanne Bruner (deanne.bruner@oregonstate.edu) on 2015-07-06T19:19:40Z No. of bitstreams: 2 SimonichStaciEnvironmentalMolecularToxicologyRelativeInfluenceTrans-Pacific.pdf: 2093385 bytes, checksum: cacc05da703959780798020d7f72cbbb (MD5) SimonichStaciEnvironmentalMolecularToxicologyRelativeInfluenceTrans-Pacific(SupportingInformation).pdf: 6448095 bytes, checksum: 86d0069afef09a4a7558a72ad3bc6d64 (MD5)

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