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Distinct broadband third-harmonic generation on a thin amorphous medium–air interface Public Deposited

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This paper was published in Optics Letters and is made available as an electronic reprint with the permission of OSA. The paper can be found at the following URL on the OSA website:  http://www.osa.org/en-us/home/. Systematic or multiple reproduction or distribution to multiple locations via electronic or other means is prohibited and is subject to penalties under law.

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  • We achieve a series of distinct broadband third-harmonic generation (THG) signals at the amorphous glass–air interface attributed to third-order and cascaded third-order nonlinear processes. A novel THG laser sideband arises from cascaded interaction between fundamental pulses and the cascaded four-wave mixing signals. The spatially separated THG sidebands with distinct spectral profiles manifest femtosecond quantum beats. Using a versatile setup with two crossing near-IR pulses temporally delayed to each other, we design an incident pulse polarization control method on the THG sideband lasers and also acquire the low-frequency surface Raman spectrum of the amorphous medium.
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  • Liu, W., Wang, L., Han, F., & Fang, C. (2013). Distinct broadband third-harmonic generation on a thin amorphous medium-air interface. Optics Letters, 38(17), 3304-3307. doi:10.1364/OL.38.003304
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  • This work was supported by the Oregon State University (OSU) faculty startup research grant and the venture fund award to C. Fang.
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