Intraexciton transitions in semiconductor quantum wells are modulated by strong and tunable few-cycle terahertz pulses. Time-resolved terahertz-pump and optical-probe measurements demonstrate that the 1s heavy-hole and light-hole exciton resonances undergo large-amplitude spectral modulations when the terahertz radiation is tuned near the 1s–2p intraexciton transition. The strong nonlinear optical transients exhibit...
Quantum mechanics provides a conventional theory of scattering that is limited in
at least two ways: it focuses exclusively on the asymptotic regime and, in a more general
sense characteristic of all quantum descriptions, provides no concrete account of individual
particle evolution in spacetime. This is particularly true during the...
We construct a quantum interchange walk, related to classical walks with memory. This gives us a coinless discrete walk, while the origin in classical walks with memory offers the promise of use of existing tools from classical memoried walks. This approach readily reproduces all standard approaches. We briefly discuss its...
Double excitonic absorption peaks are observed in textured BaCuSF and BaCuSeF thin films. The excitonic doublet separation increases with increasing fraction of heavy chalcogen in the thin-film solid solutions, in good agreement with the spin-orbit splitting of the valence bands calculated by density-functional theory. In BaCuSF and BaCuSeF, the excitons...
In situ photoemission spectroscopy experiments are used to characterize the interface between ZnTe and the wide band gap p-type semiconductor BaCuSeF. The contact is characterized by a null valence-band offset, a large conduction-band offset, and a chemically graded interface. By applying the transitivity rule for band offset and on the...
BaCuChF (Ch = S, Se, Te) materials are chalcogen-based transparent conductors with wide optical band gaps (2.9 – 3.5 eV) and a high concentration of free holes (10¹⁸ – 10²⁰ cm⁻³) caused by the presence of copper vacancies. Chalcogen vacancies compensate copper vacancies in these materials, setting the Fermi level...
BaCuChF (Ch=S,Se,Te) surfaces and BaCuSeF interfaces with zinc phthalocyanine (ZnPc) were studied by photoelectron spectroscopy. BaCuChF compounds oxidize when exposed to ambient atmosphere. Se capping layers were studied as a means to produce representative surfaces for photoelectron spectroscopic measurements. Decapped BaCuSeF surfaces remain O-free and C-free when the Se layer...
The process of de-excitation of the actinides is a very important question in both pure and applied science. In this dissertation the process was studied using the neutrons emitted in coincidence with fission induced by the bombardment of ²³⁸U with 14.85 MeV deuterons. Neutrons can be emitted at multiple stages...
This dissertation concerns several problems in the fields of light interaction with nanostructured media, metamaterials, and plasmonics. We present a technique capable of extending operational bandwidth of hyperbolic metamaterials based on interleaved highly-doped InGaAs and undoped AlInAs multilayer stacks. The experimental results confirm theoretical predictions, exhibiting broadband negative refraction response...
Native point defects, defect complexes, and oxygen impurities in BaCuChF were studied using density
functional theory calculations, self-consistent thermodynamic simulations, and various experimental techniques.
Unintentional p-type conductivity in BaCuChF is explained by the presence of copper vacancies with
transition levels in the valence band. These acceptor-like defects are partially compensated...