We report on a novel class of semiconductor metamaterials that employ a strongly anisotropic dielectric function to achieve negative refraction in the midinfrared region of the spectrum, ~8.5–13 μm. We present two types of metamaterials, layered highly doped/undoped heterostructures and quantum well superlattices that are highly anisotropic. Contrary to other...
The authors demonstrate the generation of multicycle narrow-bandwidth terahertz pulses in periodically inverted GaAs structures using optical rectification of 2 μm, 100 fs pump pulses. Three different types of orientation-inverted samples are employed: optically contacted multilayer, orientation-patterned, and diffusion-bonded GaAs. The terahertz pulses are characterized by two-color (pump at 2...
The authors demonstrate a flexible terahertz pulse-shaping technique, manipulating spatially dispersed multifrequency components generated by optical rectification in a fanned-out periodically poled lithium niobate crystal. Spatial masks of low pass, high pass, and double slit in front of the crystal manipulate the spatial pattern of the optical excitation beam on...
In this dissertation we study the electromagnetic properties of plasmonic metamaterials. We develop an analytical description to solve the fundamental problem of free-space scattering in planar plasmonic systems by utilizing anisotropic metamaterials. We show with exact numerical simulations that these manufactured materials do completely eliminate the scattering, and even in...
The ability to interpret graphical information is a prime concern in physics as
graphs are widely used to give quick summaries of data sets, for pattern recognition, and for analysis of information. While visual graphs have been developed so that their content can be readily and concisely discerned, there is...
The results of an investigation into carrier dynamics in several novel functionalized and solution-processable pentacene and anthradithiophene derivatives are reported. Measurements were made of real-time photoresponse of polycrystalline thin films of these materials to ultrafast laser pulses, on picosecond to microsecond time-scales, as well as measurements of dark current and...
In this dissertation we study the electromagnetic properties of planar waveguides
with non-magnetic strongly anisotropic dielectric cores. We develop an analytical
description of the mode propagation in these systems and show that the index
of refraction can be either positive or negative depending on the specific material
parameters. Propagating modes...
Theories predict that making a dilute magnetic semiconductor strongly p -type would allow it to remain ferromagnetic at room temperature. This is of intrest as a ferromagnetic semiconductor would allow for a great many applications in the field of spintronics. Neutron scattering experiments were undertaken to better understand the antiferromagnetic...
Aquifer recharge is generally driven by fluids that move from the Earth’s surface to groundwater through the unsaturated zone, also known as the vadose zone. When the vadose zone is fractured, fluids, which may include contaminants, can move through the fracture network as well as the porous matrix. Such a...
The main result of this written dissertation is a mathematical solution to the problem of multiplex recording for high performance tandem time-of-flight mass spectrometry. The prescription is to use a time-lag accelerator in the second stage to match the ion optical properties of the decay fragments to the requirements of...
Total electronic energies are calculated numerically for
free and singly-ionized He, Li, C, and Ne atoms using density
functional theory. Immersion energies are calculated for a single
C impurity atom embedded or absorbed into a charge-neutral system
composed of a free-electron gas with uniform positive background,
also called 'jellium'. Nonspherical...
This work comprises two main parts: creating and shaping narrowband, pulsed THz radiation in a table-top optical setup; and applying THz pulses to semiconductor nanostructures to study electron dynamics.
I developed a scheme to shape the THz output of a fanned-out periodically poled lithium niobate (PPLN) crystal. The pulses are...
This thesis deals with applications of uniaxial anisotropic crystals for microcavity resonators with partially chaotic underlying ray dynamics. We develop an implementation of the scattering matrix formalism, and relate the eigenvalues and eigenvectors of the scattering matrix to the field distribution of inside the system. Using the developed technique, we...
Gallium arsenide shows excellent promise for terahertz generation using mid infrared.
This is for two reasons. First, the indices of refraction for the terahertz (nTHz=3.61 at 1 THz) and mid infrared (nopt=3.431 at 2 μm) are close allowing a long interaction length.
Second, the linear absorption is low at terahertz...
A new, reproducible method of using electromigration to form
metallic nano-conductors is developed using gold and a tin-silver alloy.
Measurements revealed a quantization of the electrical conductance
consistent with the theory of quantum conductance. The theory of
quantum conductance is applied to show that a nano-conductor with a
cross-section of...
This dissertation concerns a broad range of unique phenomena related to the light propagation at nano- and micro-scales. To access the nano-domain, we introduce anisotropy-based waveguides with positive- and negative-index modes. These novel structures allow energy propagation in subwavelength regions and, in contrast to surface waves, have the mode structure...
In this thesis I studied several THz components that can be used for potential THz
technology. THz waves were generated in nonlinear medium via optical rectification
of femtosecond optical pulses. Utilizing the phase matching condition between the
optical and THz waves in a ZnTe crystal, single-cycle broad-band THz pulses were...
The extended-Lifshitz-Kosevitch formalism (ELK) unifies the treatment of
the de Haas-van Alphen (dHvA) effect, allowing it to transcend its traditional roles
of mapping Fermi surfaces and measuring effective masses. Here we exploit the
capabilities of dHvA as a probe of many-body effects to examine heavy-fermion su-
perconductivity. ELK successfully describes...