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Filtering by: Alternative title ssim Report no. 1704 Remove constraint Alternative title ssim: Report no. 1704 Advisor White, James D. Remove constraint Advisor: White, James D. Committee Member Blakemore, Paul Remove constraint Committee Member: Blakemore, Paul Degree Name Doctor of Philosophy (Ph.D.) Remove constraint Degree Name: Doctor of Philosophy (Ph.D.)

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  • Studies toward the total synthesis of sanglifehrin A

    Creator:
    Suttisintong, Khomson
    Abstract:
    Studies toward synthesis of subunits of sanglifehrin A, an immunosuppressant featuring a highly substituted [5,5]-spirolactam moiety as well as a 22-membered macrocycle are described. The macrolactone contains a peptidic backbone characterized by an unusual [beta]-substituted (S)-piperazic acid and (S)-m-hydroxyphenylalanine units. These studies resulted in the synthesis of advanced intermediate 358...
    Resource Type:
    Dissertation
    Full Text:
    of one less step but no increase in yield is depicted in Scheme 2.2. Subjection of propagylic