The oxidation of carbon monoxide (CO) to carbon dioxide (CO2) is ubiquitous throughout many industrial processes and is a common probe reaction used to help understand catalytic systems in research settings. The reaction is essential in power generation and transportation exhaust gas treatment technologies to ensure environmental safety, because CO...
The continued long-term use of fossil fuels as a primary energy source has resulted in dramatic increases in greenhouse gas emissions and the associated concerns of climate change and environmental pollution. A key strategy to circumvent these issues is a global shift away from fossil fuels toward renewable energy sources....
Heterogeneous catalysis modulates the rate and selectivity of reaction processes by
stabilizing a series of intermediate states on solid surfaces, facilitating the production
of many commodity chemicals modern society relies upon. Conventional, thermal
catalytic processes—conducted at elevated temperatures and pressures—source
thermal, mechanical, and chemical potential energy from carbon-hydrogen bonds—
combustion...
Water electrolysis plays a pivotal role in achieving a green hydrogen economy by sourcing electricity from intermittent renewable sources. However, the efficiency of the electrolysis process is limited by the sluggish oxygen evolution reaction (OER) kinetics, whereas the kinetics of the hydrogen evolution reaction (HER) are more facile. This thesis...
Spontaneous quasicrystal (QC) formation has not been observed in pure metals either in computation or in experiments (excluding epitaxial growth of thin atomic layers on a QC template). In this thesis work, dodecagonal QC (DDQC) grains are first discovered to spontaneously form during thermal devitrification of pure tantalum (Ta) metallic...
The continuous development of higher performing battery materials has emerged in parallel with the development of new manufacturing processes. Nanomaterials are one solution to addressing the cycling and performance challenges that limit existing battery cells. However, many of the methods used today for nanomaterial synthesis are high temperature batch methods...
The demand for the development of sustainable energy is an all time high as we burn through limited fossil fuel reserves and as environmental concerns rise every year. Renewable energy sources such as wind and solar power have limitations due to inconsistent power supply that cannot meet the regular needs...
The grand plan of carbon neutralization and COP26 in Glasgow require a quick shift of energy sources from conventional fossil fuel to a more renewable substitute such as wind, or solar energy. However, the intermittency of those renewable energy sources does not meet the demand of the energy, which requires...
Metallic glasses (MGs) have attracted tremendous attention because of their unique properties and potential applications in the future industry. However, it is still a mystery for people to understand the formation mechanism of the bulk MGs (BMGs). To produce BMGs, the specific composition of materials, sufficiently high cooling rate, etc.,...
Dense electrical recording of biosignals has been developed to provide spatial resolution and precise temporal information for health monitoring, diagnostics, and clinical research. However, more electrodes require more wires, and wiring density quickly becomes a limiting factor. To break this bottleneck, we proposed a frequency-division multiplexing (FDM) based architecture for...