We have developed a new approach to the theory of linear dichroism in partially ordered systems. The description of the partially ordered ensemble uses a density of states function, D(θ, ϕ, Δ), which gives the probability that the direction of polarization for incident polarized light has spherical angles θ and...
We have developed a method for determining the response of a static, partially ordered ensemble of molecules to various types of electromagnetic probes. In our formalism a physical model is constructued for the orientational distribution function, which is represented as a volume integral over a set of weighting functions. Procedures...
We have expanded on the results of an earlier paper [J. Chem. Phys. 72, 221 (1980)] which deals with a method for determining the response of a static, partially ordered ensemble of molecules to various types of electromagnetic probes. In this paper we consider types of spectroscopy whose response depends...
A single‐photon timing system is described which is capable of extracting fluorescence lifetimes as short as 25 ps. The system is an improved version of an earlier apparatus. The new system uses a synchronously pumped, mode‐locked dye laser with 10‐ps pulses operating at 82‐MHz repetition rate. A fast photodetector and...