Exciton polaritons are quasiparticles composed of a quantum superposition of matter and light states that arises from the coupling of a standing wave photon and an exciton. This research has two primary objectives: to design and fabricate a Fabry-Perot microcavity system in which to produce exciton polaritons; and to show...
Organic semiconductors are of interest for (opto)electronic applications due to their low cost, solution processability, and tunable properties. Natural product-derived organic pigments have attracted attention due to their extraordinary environmental stability and unexpectedly good optoelectronic performance, in spite of only partially conjugated molecular structures. Fungi-derived pigments are a naturally sourced,...
We explore the interactions between charge transfer exciton states (CTEs) and an optical microcavity by testing the effects that cavity resonance has on the CTEs and if CTEs can be coupled with a photon to create quasiparticles known as polaritons. Exciton polaritonics is becoming a booming area of research mainly...
Organic semiconducting materials have emerged in the last few decades as viable alternatives to inorganics in broad applications from field effect transistors to LEDs to solar cells. Organics provide many benefits over inorganics such as flexibility, sustainability, and reduced cost. However, these materials are more susceptible to degradation in the...
Organic semiconductors are a promising alternative to the traditional inorganic semiconductors, such as silicon. Organics are solution-processable, low-cost, sustainable, and have interesting optoelectronic properties. One such property is the formation of exciton-polaritons, quantum quasi-particles formed by an electron-hole pair in the semiconductor and a photon. This process can be induced...
The behavior and application of organic semiconductor materials depend strongly on their molecular structure, and molecular interactions. Several studies of intermolecular interactions in functionalized polyacene materials are presented. The degree and onset of aggregation of a functionalized anthradithiophene derivative was studied as a function of concentration in two different host...
The continued development of organic semiconductor materials relies on an understanding of the relationship between optoelectronic properties, molecular structure, and molecular interaction. Several detailed studies of electronic properties in functionalized polyacene materials are presented. A computational model which allows the extraction of charge generation and transport properties from experimental data...
This research investigates the electronic properties of a fungi-derived pigment, xylindein
as a novel sustainable material for organic electronics. Xylindein molecules were characterized in solution and in film. Absorption spectra and (photo)luminescence spectra were
taken at various excitation wavelengths. Xylindein’s molecular properties were computed
with the Gaussian 09 software suite....
Organic semiconductors are used in a wide variety of applications including transistors,solar cells, and light emitting diodes. These materials are solution-processable,low cost, and tunable. Many successful organic optoelectronic materials utilizeblends of several types of molecules (such as donors and acceptors) in order topromote charge generation. As blends are an inherently...